A new approach for preparing twist-type silicon bicrystals and compliant su
bstrates is reported. Thin single-crystal silicon films prepared from a sil
icon-on-insulator wafer can be bonded to each other or to silicon substrate
s. Thousands of silicon bicrystals bonded at different twist angles can be
obtained in a single preparation process and are ready for transmission ele
ctron microscopy (TEM) examination. Plan-view and high resolution cross-sec
tional TEM images of the silicon bicrystals are presented. Dislocation netw
ork and moire fringes of small-angle twist-type silicon boundaries are show
n. This technique facilitates the systematic study of small- and large-angl
e grain-boundary structures of silicon. A possible application to fabricati
ng compliant substrates for heteroepitaxial growth of Si1-xGex is discussed
.