We report on investigations of the crystallographic structure and the magne
tic anisotropies of epitaxial iron films deposited onto periodically steppe
d Ag(001) surfaces using low energy electron diffraction, x-ray diffraction
, second harmonic generation (SHG), as well as the Brillouin light scatteri
ng (BLS) technique. The focus of the present study lies on the interrelatio
n between the surface morphology of the buffer layers and the magnetic prop
erties of the Fe films, epitaxially grown onto them. Especially the symmetr
y breaking at the atomic steps is found to create an uniaxial magnetic anis
otropy measured by BLS and a very strong anisotropic signal in magnetic SHG
. (C) 2000 American Institute of Physics. [S0021-8979(00)50708-7].