Significantly enhanced anisotropic magnetoresistance (MR) in permalloy (Ni0
.81Fe0.19) films deposited on a thin (Ni0.81Fe0.19)(1-x)Cr-x or Ni1-xCrx un
derlayer is reported. The maximum Delta R/R enhancement was observed using
the underlayer with x approximate to 0.44 at an optimum thickness of approx
imate to 30-45 Angstrom, depending on the deposition technique. An enhancem
ent of 75%-150% was observed for 45-430 Angstrom thick permalloy films, com
pared to the films deposited without this underlayer. The Delta R/R enhance
ment is attributed to the decrease in the resistivity rho and the increase
in Delta rho of the permalloy film due to the formation of large (111) text
ured crystal grains in the permalloy films deposited on this underlayer, as
revealed by the x-ray diffraction results obtained using synchrotron radia
tion. (C) 2000 American Institute of Physics. [S0021-8979(00)44308-2].