Time-resolved Kerr rotation and resonant spin amplification are used to stu
dy spin dynamics in ZnSe epilayers and across a GaAs/ZnSe interface. In acc
ord with previous studies in GaAs we find that modest n doping of ZnSe epil
ayers enhances spin lifetimes over three orders of magnitude at low tempera
tures. Lifetimes reaching 60 ns are seen at low doping concentrations at te
mperatures from 5 to 50 K. A recently developed two-color technique of time
-resolved Kerr rotation is used to excite electron spins in a GaAs substrat
e and to measure their arrival in an adjacent ZnSe epilayer. We find that r
esonant spin amplification may be used to increase the net spin transferred
to the ZnSe, and discover that interlayer transport extends spin lifetimes
100-fold. (C) 2000 American Institute of Physics. [S0021-8979(00)30408-X].