Based on far-infrared spectroscopy of a small sample of nearby infrared-bri
ght and ultraluminous infrared galaxies (ULIRGs) with the ISO Long Waveleng
th Spectrometer(1) we find a dramatic progression in ionic/atomic fine-stru
cture emission line and molecular/atomic absorption line characteristics in
these galaxies extending from strong [O III]52,88 mu m and [N III]57 mu m
line emission to detection of only faint [C II]158 mu m line emission from
gas in photodissociation regions in the ULIRGs. The molecular absorption sp
ectra show varying excitation as well, extending from galaxies in which the
molecular population mainly occupies the ground state to galaxies in which
there is significant population in higher levels. In the case of the proto
typical ULIRG, the merger galaxy Arp 220, the spectrum is dominated by abso
rption lines of OH, H2O, CH, and [O I]. Low [O III]88 mu m line flux relati
ve to the integrated far-infrared flux correlates with low excitation and d
oes not appear to be due to far-infrared extinction or to density effects.
A progression toward soft radiation fields or very dusty H II regions may e
xplain these effects.