We envisage the enhanced effect of harmonic generations from aperiodic opti
cal superlattices (AOSs) achieved by inverting poled ferroelectric domains
in samples. The search of optimal AOSs structures belongs to solving a diff
icult inverse source problem in nonlinear optics. We employ the simulated a
nnealing method to successfully deal with this problem. We present the anal
yses of the design idea in the real-space representation and carry out seve
ral model designs. The constructed AOSs implement multiple wavelength secon
d-harmonic generation and the coupled third-harmonic generation with an ide
ntical effective nonlinear coefficient at the preassigned wavelengths. The
simulations show that the harmonic generations in the constructed AOSs can
approach the prescribed goal better than those with the Fibonacci optical s
uperlattice. The effective nonlinear coefficients versus the optical wave p
ropagating distance from the impinging surface of incident light in the sam
ple exhibit monotonically increasing behavior. This clearly infers that the
contribution from each and every block to the optical parametric processes
is in the constructive interference state. We also investigate the influen
ce of the random fluctuation of the thickness of blocks on the performance
of the constructed AOSs in detail for simulating practical fabrications and
testing the performance stability of the sample. (C) 2000 American Institu
te of Physics. [S0021-8979(00)00511-9].