Y. Fukaya et al., Dynamic change in the surface and layer structures during epitaxial growthof Si on a Si(111)-7X7 surface, PHYS REV B, 61(19), 2000, pp. 13000-13004
In order to investigate the dynamic process during growth of a Si layer on
the Si(111)-7 X 7 surface held at 380 degrees C, the rocking curve of refle
ction high-energy electron diffraction (RHEED) is continuously measured at
0.5 degrees to 6 degrees at intervals of 0.05 degrees to the glancing angle
of the incident electron beam which takes 18 sec. At the initial growth st
age, the multilayer islands are grown on the native 7 X 7 surface with broa
der Bragg peaks in the rocking curve than those from the native surface. Th
e sharpness of the Bragg peak is subsequently recovered after the thickness
of the Si layer reaches 3 BL (1 BL = 0.31 nm), at which the growth transfo
rms to layer-by-layer growth. The comparison of the measured rocking curve
with the calculated one based on the dynamical theory of RHEED intensity is
also performed by optimizing each atomic position in the growing layer so
as to minimize the difference between both curves. The space of the double
layer of the (111) plane in the multilayer islands expands and is restored
to the normal spacing after the growth mode transforms to the layer-by-laye
r mode. The broadening of the Bragg peaks at the initial growth stage relat
es to the rearrangement process of a stacking-fault layer in the 7 X 7 stru
cture on the substrate surface.