D. Mazzotti et al., Difference-frequency generation in PPLN at 4.25 mu m: an analysis of sensitivity limits for DFG spectrometers, APP PHYS B, 70(6), 2000, pp. 747-750
We report difference-frequency generation (DFG) in periodically poled lithi
um niobate (PPLN) around 4.25 mu m using a cw Nd:YAG and an injection-locke
d diode laser. This system provides a narrow linewidth source at 4.25 mu m
with near-shot-noise-limited operation. A conversion efficiency close to th
e theoretical limit is obtained. Detection of CO2 absorption spectra is dem
onstrated and further improvements and applications to high sensitivity spe
ctroscopy are discussed.