Aa. Gippius et al., Magnetic flux dynamics and structural features in fluorinated HgBa2CuO4 asprobed by F-19 NMR, PHYS REV B, 61(21), 2000, pp. 14370-14373
F-19 NMR spectra and spin-lattice relaxation rates have been measured on tw
o powder HgBa2CuO4Fx samples. The results combined with our neutron powder-
diffraction data [A. M. Abakumov rt al., Phys. Rev. Lett. 80, 385 (1998)] c
onfirm that fluorine atoms can be successfully incorporated in the lattice
of superconducting Hg-1201 phase in the nonstoichiometric O3 site. Partial
occupation of another oxygen position by fluorine atoms reveals to be possi
ble with the increase of F content. The temperature dependence of the F-19
NMR linewidth reveals the crossover at 35 K in the magnetic-flux line struc
ture between the low-temperature latticelike regime and high-temperature "m
elted" regime. For the 1/T-1 temperature dependence a maximum has been foun
d at 65 K indicating the strong influence of magnetic-flux line motion on t
he F-19 spin-lattice relaxation rate.