We report on single-pass optical gain measurements in poly(styrene) wavegui
des doped with polymeric model compounds under picosecond excitation. Using
a wavelength-dependent model of amplified spontaneous emission, we produce
optical gain spectra for these materials. Large net optical gains are prod
uced for small input pulse energies. A figure of merit describing the poten
tial of a material for use as a laser medium is presented. Comparisons with
other recent publications indicate that organic materials can compete with
inorganic semiconductors for optically pumped applications. (C) 2000 Elsev
ier Science S.A. All rights reserved.