Investigations have been performed on harmonic generation from solid-vacuum
interfaces using a 2,2-ps 1054-nm laser pulse at maximum intensities of si
milar to 2x10(17) W . cm(-2). It is found that the divergence of the harmon
ics gradually increases at intensities between I lambda(2) = 2 x 10(15) and
2 x 10(16) W cm(-2) . mu m(2). We experimentally observe that the divergen
ce of cm the harmonics decreases as the order of the harmonic increases. We
also found that the divergence of the third harmonics emission is smaller
for 2,2-ps pulsewidth for the driving lasers as compared with those for 100
-ps pulsewidth lasers.