B. Doliwa et A. Heuer, Cooperativity and spatial correlations near the glass transition: Computersimulation results for hard spheres and disks, PHYS REV E, 61(6), 2000, pp. 6898-6908
We examine the dynamics of hard spheres and disks at high packing fractions
in two and three dimensions, modeling the simplest systems exhibiting a gl
ass transition. As it is well known, cooperativity and dynamic heterogeneit
y arise as central features when approaching the glass transition from the
liquid phase, so an understanding of their underlying physics is of great i
nterest. Cooperativity implies a reduction of the effective degrees of free
dom, and we demonstrate a simple way of quantification in terms of the stre
ngth and the length scale of dynamic correlations among different particles
. These correlations are obtained for different dynamical quantities X-i(t)
that an constructed from single-particle displacements during some observa
tion time t. Of particular interest is the dependence on t. Interestingly,
for appropriately chosen X-i(t) we obtain finite cooperativity in the limit
t-->infinity.