We present the first experimental evidence confirming the theoretical predi
ctions of alpha buckets in an electron storage ring. By controlling both th
e first- and second-order momentum compaction factors. we succeeded in stor
ing electrons simultaneously in a pair of alpha buckets or in either bucket
alone. The two electron bunches are separated in energy by slightly less t
han 1% and thr energy is unable over a narrow range. The energy difference
was directly measured using synchrotron light from an undulator. Simultaneo
us two-color light beams from an undulator were generated. By changing thc
rf voltage, we were able to vary the normally fixed longitudinal bunch sepa
ration.