The rotational transitions of carbon monoxide (CO) are the primary means of
investigating the density and velocity structure of the molecular interste
llar medium. Here we study the lowest four rotational transitions of CO tow
ard high-latitude translucent molecular clouds (HLCs). We report new observ
ations of the J = (4-3), (2-1), and (1-0) transitions of CO toward eight hi
gh-latitude clouds. The new observations are combined with data from the li
terature to show that the emission from all observed CO transitions is line
arly correlated. This implies that the excitation conditions that lead to e
mission in these transitions are uniform throughout the clouds. Observed (C
O)-C-13/(CO)-C-12 (1_0) integrated intensity ratios are generally much grea
ter than the expected abundance ratio of the two species, indicating that t
he regions that emit (CO)-C-12 (1-0) radiation are optically thick. We deve
lop a statistical method to compare the observed line ratios with models of
CO excitation and radiative transfer. This enables us to determine the mos
t likely portion of the physical parameter space that is compatible with th
e observations. The model enables us to rule out CO gas temperatures greate
r than similar to 30 K, since the most likely high-temperature configuratio
ns are 1 pc-sized structures aligned along the line of sight. The most prob
able solution is a high-density and low-temperature (HDLT) solution, with v
olume density, n=10(4.5+/-0.5) cm(-3), kinetic temperature, T-k approximate
to 8 K, and CO column density per velocity interval N-CO/Delta V. = 10(16.
6+/-0.3) cm(-2)/(km s(-1)). The CO cell size is L similar to 0.01 pc (simil
ar to 2000 AU). These cells are thus tiny fragments within the similar to 1
00 times larger GO-emitting extent of a typical high-latitude cloud. We dis
cuss the physical implications of HDLT cells, and we suggest ways to test f
or their existence.