A review of recent experimental and theoretical studies devoted to new acti
ve media of nuclear-pumped lasers using transitions of chlorine, carbon, ni
trogen, and oxygen atoms is provided. Optimal parameters of lasing are pres
ented, and dependences of optimal and threshold characteristics of these la
sers on the composition of the active medium are analyzed. The mechanisms b
ehind population inversion for the transitions under study are described. T
he influence of impurities on lasing through transitions of chlorine atoms
is investigated. The experimental results are analyzed in terms of comprehe
nsive nonstationary kinetic models. A list of estimates on rate constants o
f plasma-chemical reactions is presented.