We report Raman scattering from CdSe/ZnSe self-assembled quantum dot struct
ures. A series of samples, each with a different growth-interruption time b
efore ZnSe caping of the CdSe dots, is investigated. ZnSe longitudinal opti
cal (LO) phonon shifts as a function of the interruption time show a comple
x pattern due to the evolution of CdSe dots. We observe an LO phonon from t
he CdSe dots at similar to 221 cm(-1) as well as an interface phonon at sim
ilar to 245 cm(-1). We present evidence that the interface phonon is locali
zed at the interface between the CdSe dots and the ZnSe cap layer.