We demonstrate the possibility of growing good-quality epitaxial Fe films o
n a Si(001) substrate, opening up new prospects to prepare ferromagnetic su
perlattices on this substrate. A template technique prevents the formation
of disordered interfacial iron silicides. Transmission electron microscopy
reveals that the Fe layers are fairly uniform in thickness with abrupt inte
rfaces and in majority epitaxial relationship Fe(001)[100]//Si(001)[100]. B
oth the diffraction data and the observation of Moire fringes indicate that
the Fe lattice is almost relaxed towards its bulk bcc phase in thick layer
s [greater than or equal to 40 monolayers (ML)] but is still strained by th
e substrate in the thinnest films. Magneto-optical Kerr effect measurements
show that the films evaporated at normal incidence with a thickness above
4 ML are ferromagnetic at room temperature and exhibit in-plane biaxial ani
sotropy. (C) 2000 Elsevier Science B.V. All rights reserved.