Resonant and non-resonant ionization of helium by XUV ultrashort and intense laser pulses

Citation
R. Hasbani et al., Resonant and non-resonant ionization of helium by XUV ultrashort and intense laser pulses, J PHYS B, 33(11), 2000, pp. 2101-2116
Citations number
33
Categorie Soggetti
Physics
Journal title
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS
ISSN journal
09534075 → ACNP
Volume
33
Issue
11
Year of publication
2000
Pages
2101 - 2116
Database
ISI
SICI code
0953-4075(20000614)33:11<2101:RANIOH>2.0.ZU;2-E
Abstract
We study the multiphoton ionization of He by a strong ultrashort laser puls e. We solve the time-dependent Schrodinger equation numerically by means of a spectral method of configuration-interaction type (CI). Our method is ba sed on an expansion on B-spline functions, more precisely each two-electron configuration is built as an antisymmetrized B-spline product for the (two -dimensional) radial part and dipolar spherical harmonics for the (four-dim ensional) angular part. We focus on both the atomic structure calculations and the laser-atom dynamics. We show that our approach allows one to proper ly treat the electron-electron correlations so as to provide an accurate de scription of many eigenstates simultaneously The method is applied in two d ifferent situations: (a) the multiphoton excitation and ionization of heliu m with photon energies ranging from 5.4 to 32.6 eV and (b) the two-photon i onization of helium below the He+(2l) threshold and three-photon ionization above the He2+ threshold with photon energies ranging from 25.8 to 34 eV. The results are compared with other CI calculations (where a comparison is possible) and, in case (a), tb Hartree-Fock calculations. In case (b) we pa rticularly focus on the dynamics of the production of doubly-excited struct ure by laser pulses with a duration which is shorter than the autoionizatio n lifetime.