Muon-spin rotation (mu SR) measurements have been used to study the superco
nducting vortex properties of the organic superconductors kappa-(BEDT-TTTF)
(2) Cu(SCN)(2), alpha-(BEDT-TTF)(2) NH4Hg(SCN)(4) and beta-(BEDT-TTF)(2)IBr
2. These materials all have highly anisotropic structures consisting of met
allic layers of BEDT-TTF molecules alternating with less well conducting an
ion layers. Varying the anion gives rise to a change in the anisotropy of t
he superconductivity and also to changes in the superconducting transition
temperature. We have used both transverse and longitudinal magnetic fields
to study the three-dimensional flux line lattice that is present at low tem
peratures and fields and to study also the loss of flux lattice order that
occurs on increasing the temperature and field. (C) 2000 Elsevier Science B
.V. All rights reserved.