The effects of surface modification on the magnetic properties of polymer-b
onded Nd-Fe-B magnets have been studied. Two sets of Nd-Fe-B powders, coate
d and uncoated, were blended and compression molded with polyphenylene sulf
ide in isotropic form. Their magnetic properties were measured using a Helm
holtz coir and a SQUID. The results showed that the effect of the coating s
ignificantly improved the irreversible loss in flux and energy product of t
he polymer-bonded magnets. The results have been interpreted using an isotr
opic model of hysteresis that takes into account energy losses. The modelin
g showed that the presence of soft magnetic materials in the Nd-Fe-B powder
s caused by oxidation reduces the interaction among magnetic particles, how
ever, the coating treatment alters the magnetic properties by increasing th
e remanence of polymer-bonded magnets via increasing the interparticle coup
ling coefficient. (C) 2000 Elsevier Science B.V. All rights reserved.