Structural and magnetic properties of the two-layered Ruddlesden-Popper pha
se SrO(La1-xSrxMnO3)(2) with x=0.3-0.5 are highlighted. Intrinsic propertie
s of these naturally layered manganites include a "colossal" magnetoresista
nce, a composition-dependent magnetic anisotropy, and almost no remanence.
Above the Curie temperature there is a nonvanishing extrinsic magnetization
attributed to intergrowths (stacking faults in the layered structure). The
se lattice imperfections consist of additional or missing manganite lagers,
as observed in transmission electron microscopy. Their role in influencing
the properties of the host material is highlighted. (C) 2000 American Vacu
um Society, [S0734-2101(00)01404-4].