We report on electrically driven amplified spontaneous emission and Lasing
in tetracene single crystals using field-effect electrodes for efficient el
ectron and hole injection. For Laser action, feedback is provided by reflec
tions at the cleaved edges of the crystal resulting in a Fabry-Perot resona
tor. Increasing the injected current density above a certain threshold valu
e results in the decreasing of the spectral width of the emission from 120
millielectron volts to Less than 1 millielectron volt because of gain narro
wing and eventually Laser action. High electron and hole mobilities as well
as balanced charge carrier injection Lead to improved exciton generation i
n these gate-controlled devices. Moreover, the effect of charge-induced abs
orption is substantially reduced in high-quality single crystals compared w
ith amorphous organic materials.