Fine-particle emissions of energy production in Finland

The aim of this study was to find out the fine-particle emissions (PM2.5) o f different energy production processes in Finland. The main purpose was to compare the calculated emission factors between different energy productio n concepts. The purpose was also to define what is known about fine-particl e emissions and what should still be studied/measured. Only those energy pr oduction processes that produce a significant amount of direct emissions of solid particles have been treated here, i.e. pulverized combustion and oil burners from burner combustion, fluidized bed combustion processes, grate boilers, recovery boilers and diesel power plants. Secondary particles from gaseous pollutants have not been considered within this study. In pulveriz ed coal combustion the particle emission is composed mainly of particles sm aller than 5 mu m in aerodynamic diameter. Roughly half of the total mass o f particle emission is composed of fine particles (PM2.5). Depending on boi ler size category and particle separation devices, the specific emission fa ctor for fine particles is 1-30 mg MJ(-1). For pulverized combustion of pea t, ca. 20-25% of the total mass of particle emission is fine particles, and then the specific emission factor is between 5 and 8 mg MJ(-1). For recove ry boilers, the fine particle portion of the total particle emission is 50- 60% (by mass) and the specific emission factor for fine particles varies co nsiderably according to the boiler size category, being between 12 and 77 m g MJ(-1). For oil burners, grate boilers and fluidized bed combustion proce sses, the fine-particle portion of the total particle emission could not be determined, because there were no applicable measurement results at hand. For these combustion techniques, more public measurements are needed in ord er to clarify the amount and composition of fine particles with different f uel varieties. Additionally, the chemical composition of fine particles is a very important feature when human health effects caused by particulate ma tter are considered. (C) 2000 Elsevier Science Ltd. All rights reserved.