Yk. Yoo et al., Room-temperature electronic phase transitions in the continuous phase diagrams of perovskite manganites, NATURE, 406(6797), 2000, pp. 704-708
Highly correlated electronic systems-such as transition-metal oxides that a
re doped Mott insulators-are complex systems which exhibit puzzling phenome
na, including high-temperature superconductivity and colossal magnetoresist
ivity. Recent studies(1-3) suggest that in such systems collective electron
ic phenomena are important, arising from long-range Coulomb interactions an
d magnetic effects. The qualitative behaviour of these systems is strongly
dependent on charge filling (the level of doping) and the lattice constant.
Here we report a time-efficient and systematic experimental approach for s
tudying the phase diagrams of condensed-matter systems. It involves the con
tinuous mapping of the physical properties of epitaxial thin films of perov
skite manganites (a class of doped Mott insulator) as their composition is
varied. We discover evidence that suggests the presence of phase boundaries
of electronic origin at room temperature.