Role of unstable directions in the equilibrium and aging dynamics of supercooled liquids

Citation
C. Donati et al., Role of unstable directions in the equilibrium and aging dynamics of supercooled liquids, PHYS REV L, 85(7), 2000, pp. 1464-1467
Citations number
33
Categorie Soggetti
Physics
Journal title
PHYSICAL REVIEW LETTERS
ISSN journal
00319007 → ACNP
Volume
85
Issue
7
Year of publication
2000
Pages
1464 - 1467
Database
ISI
SICI code
0031-9007(20000814)85:7<1464:ROUDIT>2.0.ZU;2-Q
Abstract
The connectivity of the potential energy landscape in supercooled atomic li quids is investigated through a calculation of the instantaneous normal mod es spectrum and a detailed analysis of the unstable directions in configura tion space. We confirm the hypothesis that the mode-coupling critical tempe rature is the T at which the dynamics crosses over from free to activated e xploration of configuration space. We also observe changes in the local con nectivity of configuration space sampled during aging, following a temperat ure jump from a liquid to a glassy state.