The effects of anthropogenic particulate emissions from ships on the radiat
ive, microphysical, and chemical properties of moderately polluted marine s
tratiform clouds are examined. A case study of two ships in the same air ma
ss is presented where one of the vessels caused a discernible ship track wh
ile the other did not. In situ measurements of cloud droplet size distribut
ions, liquid water content, and cloud radiative properties, as well as aero
sol size distributions (outside cloud, interstitial, and cloud droplet resi
dual particles) and aerosol chemistry, are presented. These are related to
measurements of cloud radiative properties. The differences between the aer
osol in the two ship plumes are discussed; these indicate that combustion-d
erived particles in the size range of about 0.03-0.3-mu m radius were those
that caused the microphysical changes in the clouds that were responsible
for the ship track.
The authors examine the processes behind ship track formation in a moderate
ly polluted marine boundary layer as an example of the effects that anthrop
ogenic particulate pollution can have in the albedo of marine stratiform cl
ouds.