The paper studies the possibility of simultaneous determination of the vert
ical characteristics of temperature, moisture and ozone content based on gr
ound measurements of downwelling thermal IR radiation in the region of the
absorption bands for CO2 (15 mu m), O-3 (9 S mu m) and H2O (6.3 mu m). Meas
uring apparatus of the Fourier-interferometer type with spectral resolution
of the order of 0.25-1.0 cm(-1) in the 4-18 mu m measurement region is con
sidered. It is shown that in conditions of a cloud-free atmosphere, the err
or in determination of total ozone is 3.5-5.5%, for total moisture 2-4%, fo
r tropospheric ozone 8-12% and for moisture in the lower troposphere 2-3%.