Homogeneous line-width of optical transitions and multiple electron-LO-phonon scattering in quantum dots

Citation
K. Kral et al., Homogeneous line-width of optical transitions and multiple electron-LO-phonon scattering in quantum dots, J CHIN CHEM, 47(4A), 2000, pp. 753-757
Citations number
11
Categorie Soggetti
Chemistry
Journal title
JOURNAL OF THE CHINESE CHEMICAL SOCIETY
ISSN journal
00094536 → ACNP
Volume
47
Issue
4A
Year of publication
2000
Pages
753 - 757
Database
ISI
SICI code
0009-4536(200008)47:4A<753:HLOOTA>2.0.ZU;2-S
Abstract
The optical line-shape of electronic transitions due to the polar electron- LO-phonon interaction in semiconductor quantum dots is studied. The mechani sm of the finite optical line-width is based on the multiple electron-LO-ph onon scattering. The influence of the higher order corrections beyond the s elf-consistent Hartree-Fock approximation to the electron-phonon part of th e electronic self-energy is estimated quantitatively. The problem is studie d within the two-level model of a single electron interacting with the syst em of longitudinal optical phonons of the whole bulk sample of the polar se miconductor. The influence of the higher order corrections is demonstrated on the line-shape of the optical transitions, the temperature dependence of the line-width and on the dependence of the line-width on the size of the quantum dot.