K. Kral et al., Homogeneous line-width of optical transitions and multiple electron-LO-phonon scattering in quantum dots, J CHIN CHEM, 47(4A), 2000, pp. 753-757
The optical line-shape of electronic transitions due to the polar electron-
LO-phonon interaction in semiconductor quantum dots is studied. The mechani
sm of the finite optical line-width is based on the multiple electron-LO-ph
onon scattering. The influence of the higher order corrections beyond the s
elf-consistent Hartree-Fock approximation to the electron-phonon part of th
e electronic self-energy is estimated quantitatively. The problem is studie
d within the two-level model of a single electron interacting with the syst
em of longitudinal optical phonons of the whole bulk sample of the polar se
miconductor. The influence of the higher order corrections is demonstrated
on the line-shape of the optical transitions, the temperature dependence of
the line-width and on the dependence of the line-width on the size of the
quantum dot.