A technique to reduce charge transfer has been studied to cut enrichment lo
ss during atomic vapor laser isotope separation. The charge transfer cross
sections of uranium R-ere experimentally examined. The cross sections of ch
arge transfer for case A (between ground-state ions and atoms) and, cases B
and C (between ions populated in some excited states and atoms) were relat
ively measured in the energy range of 100 2,000 eV by the cross-beam method
. The charge transfer cross sections for cases A, B and C do not depend on
impact energy, and the cross sections for case A are smaller than those for
cases B and C. These results are in fairly good agreement agreed with theo
retical predictions. It is confirmed experimentally and theoretically that
the uranium charge transfer cross section depends on its initial ionic stat
e, therefore ion loss by charge transfer will be reduced by controlling the
initial state of the ions.