Vm. Churikov et Cc. Hsu, Optical control of third-harmonic generation in azo-doped polymethylmethacrylate thin films, APPL PHYS L, 77(14), 2000, pp. 2095-2097
The possibility of controlling third-harmonic generation in polymethylmetha
crylate doped with disperse red 1 via exposition by frequency-doubled and f
undamental radiation of a Nd:YAG laser is demonstrated. It was possible to
change the third-harmonic efficiency up to four times depending on pumping
intensity. The change was completely reversible after 15 min of dark relaxa
tion in the case of pumping the sample with the second harmonic. This effec
t is attributed to the reversible change of third-order susceptibility due
to trans-to-cis isomerization of azo-bond molecules. (C) 2000 American Inst
itute of Physics. [S0003-6951(00)02840-0].