An investigation was carried out on thin permanent phase polarization grati
ngs recorded in Langmuir-Blodgett films using two orthogonal circularly pol
arized Ar-ion laser beams. The films are composed of amphiphilic azo-dye mo
lecules and manifest an extremely large value of photoinduced optical aniso
tropy, Delta n approximate to 0.36. The experimental results are in excelle
nt accord with the theoretical model based on the Jones matrix representati
on of the polarization pattern. The gratings are stable at least, for half
a year. (C) 2000 American Institute of Physics. [S0003-6951(00)04236-4].