The nucleosynthesis of Be and B by spallation processes provides unique ins
ight into the origin of cosmic rays. Namely, different spallation schemes p
redict sharply different trends for the growth of LiBeB abundances with res
pect to oxygen. "Primary" mechanisms predict BeB proportional to O and are
well motivated by the data if O/Fe is constant at low metallicity. In contr
ast, "secondary" mechanisms predict BeB proportional to O-2 and are consist
ent with the data if O/Fe increases toward low metallicity as some recent d
ata suggest. Clearly, any primary mechanism, if operative, will dominate ea
rly in the history of the Galaxy. In this paper, we fit the BeB data to a t
wo-component scheme which includes both primary and secondary trends. In th
is way, the data can be used to probe the period in which primary mechanism
s are effective. We analyze the data using consistent stellar atmospheric p
arameters based on Balmer line data and the continuum infrared flux. Result
s depend sensitively on Population II O abundances (and O/Fe trends), which
have recently seen renewed interest. We explore the implications of these
results phenomenologically, using a systematic and consistent compilation a
nd fitting of BeBOFe data. Two-component Be-O fits indicate that primary an
d secondary components contribute equally at [O/H](eq) = -1.8 for Balmer li
ne data; and [O/H](eq) = -1.4 to -1.8 for IRFM. We apply these constraints
to recent models for LiBeB origin. The Balmer line data do not show any evi
dence for primary production. On the other hand, the IRFM data do indicate
a preference for a two-component model, such as a combination of standard G
CR and metal-enriched particles accelerated in superbubbles. These conclusi
ons rely on a detailed understanding of the abundance data including system
atic effects which may alter the derived O-Fe and BeB-Fe relations.