Local optical spectroscopy of semiconductor nanostructures in the linear regime

Citation
O. Mauritz et al., Local optical spectroscopy of semiconductor nanostructures in the linear regime, PHYS REV B, 62(12), 2000, pp. 8204-8211
Citations number
27
Categorie Soggetti
Apllied Physucs/Condensed Matter/Materiales Science
Journal title
PHYSICAL REVIEW B
ISSN journal
01631829 → ACNP
Volume
62
Issue
12
Year of publication
2000
Pages
8204 - 8211
Database
ISI
SICI code
0163-1829(20000915)62:12<8204:LOSOSN>2.0.ZU;2-Y
Abstract
We present a theoretical approach to calculate the local absorption spectru m of excitons confined in a semiconductor nanostructure. Using the density- matrix formalism, we derive a microscopic expression for the nonlocal susce ptibility, both in the linear and nonlinear regimes, which includes a three -dimensional description of electronic quantum states and their Coulomb int eraction. The knowledge of the nonlocal susceptibility allows us to calcula te a properly defined local absorbed power, which depends on the electromag netic field distribution. We report on explicit calculations of the local l inear response of excitons confined in single and coupled T-shaped quantum wires with realistic geometry and composition. We show that significant int erference effects in the interacting electron-hole wave function induce new features in the space-resolved optical spectra, particularly in coupled na nostructures. When the spatial extension of the electromagnetic held is com parable to the exciton Bohr radius, Coulomb effects on the local spectra mu st be taken into account for a correct assignment of the observed features.