Atmospheric aerosols were sampled from aircraft at various levels over Riha
nd in northern India during the monsoon season of 1974 and at surface level
s at Calcutta, Delhi, Varanasi and Jodhpur during different seasons of 1970
and 1971. Millipore filter assembly was used for this purpose. Chloride nu
clei, total aerosol and ice nuclei concentrations were evaluated from milli
pore filters. At Rihand/Varanasi, during the monsoon, the chloride size spe
ctrum was broader and the distribution bimodal at cloud base level while th
e spectra were narrower and the distributions unimodal at other levels. At
Rihand, chloride mass and larger giant chloride number were considerably hi
gher, total aerosol higher while ice nuclei concentrations were lower on th
e days with moderate rain as compared to those with light rain. Calcutta (m
aritime) showed maximum while Varanasi (well-inland) showed minimum chlorid
e number concentrations. As compared with Calcutta, Delhi (continental) had
lower chloride and total aerosol, and markedly higher ice nuclei concentra
tions. Varanasi (high rainfall region) showed all the values, except for sm
all-sized chlorides, notably higher with respect to Jodhpur (low rainfall r
egion). Ice nuclei concentration was lowest in winter and highest in summer
at Delhi. Variations of the aerosols during different parts of the day/nig
ht are also discussed.