Magnetorheological (MR) fluids constitute examples of controllable ("smart"
) fluids, whose rheological properties vary in response to an applied magne
tic field. These fluids typically consist of micron-sized, magnetizable par
ticles dispersed in a nonpermeable carrier fluid. The essential characteris
tic of MR fluids is that they may be continuously and reversibly varied fro
m a state of free flowing liquids in the absence of an applied magnetic fie
ld to that of stiff semi-solids in a moderate field. Understanding the magn
etic properties of MR fluids is crucial to the design of MR fluid-based dev
ices and it also provides valuable insight into the character of the micros
tructure responsible for their field-dependent rheology. Prediction of the
overall magnetic properties of MR composites is a challenging task, however
, due to the highly nonlinear and strongly spatially variable nature of the
magnetization of the constituents. In this paper we propose a model for th
is behavior that is based on the mathematical theory of homogenization. We
derive effective equations that govern the magnetic response of(periodicall
y arranged) particle-chains through magnetic saturation. Comparisons of num
erical results for these equations with experimental data show good agreeme
nt which suggests that our approach could be useful in the design of improv
ed MR fluids.