The scintillation efficiency of NaI(Tl) crystals, containing Tl concentrati
on of 0.01, 0.07 and 0.22 mole%, has been measured under electron, alpha pa
rticle and fission fragment excitations. The purpose of this program was to
provide a critical test of previously proposed models of the scintillation
process in activated alkali halides. It is found that the shape of the sci
ntillation efficiency versus dE/dx: for the three different Tl concentratio
ns is dependent on Tl concentration. The measured scintillation efficiency
is compared with the scintillation models for thallium-activated alkali hal
ides proposed by Birks, and Murray and Meyer.