The authors used a Wilson expansion cloud chamber to measure binary homogen
eous nucleation rates for pure n-octane, pure i-octane, and 3:1, 1:1, 1:3 (
mole ratio) mixtures in a temperature range from 215 to 260 K. The nucleati
on rates range from approximately 100 to 50 000 drops/cm(3) s. Current bina
ry nucleation theory is unable to predict the data for this nearly ideal sy
stem. (C) 2000 American Institute of Physics. [S0021-9606(00)51041-1].