An aromatic copolyester thermotropic liquid crystal polymer (LCP) fabric wa
s used to reinforce a polyimide (PI) matrix to produce composites. The LCP/
PI composite was made to eliminate directional difference in the mechanical
properties of LCP by controlling the individual reinforcement fabric align
ment in different directions without losing any mechanical properties. As a
result, a transversely isotropic LCP composite material could be obtained
from the highly anisotropic LCP fiber. Interfacial adhesion between the LCP
and polyimide was greatly improved by a NH3/H-2 plasma treatment on the LC
P fabric, thereby the significantly improving mechanical properties of the
composite. Moreover, inter-laminar shear strength of the LCP/PI composite w
as further increased after heat treatment at 220 degreesC for 1 hour. The L
CP/polyimide composite retains stable mechanical properties up to 250 degre
esC.