Analysis of adiabatic population transfer in multilevel systems by Huckel model

Citation
Y. Ohta et al., Analysis of adiabatic population transfer in multilevel systems by Huckel model, INT J QUANT, 80(4-5), 2000, pp. 1068-1075
Citations number
28
Categorie Soggetti
Physical Chemistry/Chemical Physics
Journal title
INTERNATIONAL JOURNAL OF QUANTUM CHEMISTRY
ISSN journal
00207608 → ACNP
Volume
80
Issue
4-5
Year of publication
2000
Pages
1068 - 1075
Database
ISI
SICI code
0020-7608(200011/12)80:4-5<1068:AOAPTI>2.0.ZU;2-#
Abstract
We applied our pictorial approach using the fundamental concept of the Huck el molecular orbital theory to the population inversion in the multilevel s ystems by the straddling-STIRAP (S-STIRAP). We showed that the mechanism of the population inversion in the multilevel system may be easily understood by our approach. It is also shown that our approach is useful to understan d that the condition required for the laser frequency in the delayed pulse sequence is different for the even- and odd-level systems. (C) 2000 John Wi ley & Sons, Inc.