We present a technique for single-beam measurement of the optical nonlinear
ity in GaAs for photon energies above the bandgap. We measured the real and
the imaginary parts of the nonlinear refractive index of a bulk crystal by
using the change in reflection of dye laser pulses (10 ns, 538 nm). The va
lues obtained, n(2) = (7.8 +/- 0.6) x 10(-8) cm(2)/W and kappa (2) = (-2.8
+/- 0.7) x 10(-8) cm(2)/W, are discussed. (C) 2000 Optical Society of Ameri
ca OCIS codes: 190.4350, 190.3270.