Measurement of keV-neutron capture cross sections and capture gamma-ray spectra of Ce-140 and Pr-141

Citation
S. Harnood et al., Measurement of keV-neutron capture cross sections and capture gamma-ray spectra of Ce-140 and Pr-141, J NUC SCI T, 37(9), 2000, pp. 740-749
Citations number
47
Categorie Soggetti
Nuclear Emgineering
Journal title
JOURNAL OF NUCLEAR SCIENCE AND TECHNOLOGY
ISSN journal
00223131 → ACNP
Volume
37
Issue
9
Year of publication
2000
Pages
740 - 749
Database
ISI
SICI code
0022-3131(200009)37:9<740:MOKCCS>2.0.ZU;2-E
Abstract
The neutron capture cross sections and capture gamma -ray spectra of Ce-140 and Pr-141 were measured in the neutron energy region of 10 to 100 keV and at 550 keV. Prompt gamma rays from a capture sample were detected with a l arge anti-Compton NaI(TI) spectrometer, employing a neutron time-of-Right m ethod with a 1.5-ns pulsed neutron source by the Li-7(p, n)Be-7 reaction. A pulse-height weighting technique was applied to observed capture T-ray pul se-height spectra to extract capture yields. The capture cross sections wer e derived with the error of about 5% by using the standard capture cross se ctions of Au-197. The present results were compared with evaluated values i n JENDL-3.2 and previous measurements. The capture gamma -ray spectra were obtained by unfolding the observed capture gamma -ray pulse-height spectra. An anomalous bump was observed around 1.5 MeV in each gamma -ray spectrum of Ce-140 and Pr-141, and its energy position was consistent with the syste matics obtained in our previous work. The multiplicities of the observed ca pture gamma rays were derived from the gamma -ray spectra.