A series of NLO chromophores based on alkylamine-substituted Indole ring we
re synthesized by varying the strength of electron-acceptor. Photorefractiv
e composites consisted of carbazole-substituted polysiloxane as photoconduc
ting host, doped with prepared NLO molecules and photosensitizer. Electro-o
ptic and photorefractive properties of composites were discussed.