Charge transport in monocrystalline lead sulfide (PbS) nanoparticle films i
s investigated by current noise measurements. Monocrystalline and single-si
zed PbS nanoparticles are synthesized via the gas phase and deposited elect
rostatically onto semiconducting (GaAs) and on isolating (SiNx) substrates
with planar electrode contacts. The particles form inhomogeneous films. Low
-frequency current noise of 1-ML-thick films are measured at various voltag
es, exhibiting diffusion noise characteristics, which indicates a random-wa
lk (diffusion) phenomenon of electrons between the particles. (C) 2000 Amer
ican Institute of Physics. [S0003-6951(00)03747-5].