Chernobyl derived Cs-137 present in upper soil layers can still remain avai
lable to cation exchange and hence to downward migration. More than its phy
sico-chemical deposit forms (fuel particles and/or condensed aerosols), rad
iocesium mobility is influenced by soil properties. Although all the soils
studied contain illitic clay minerals, different Cs-137 fixation levels wer
e observed due to: (1) the reactivity state of sorption sites with a low ra
diocesium content in soil, and (2) the presence, or absence, of organic mat
ter complexes inhibiting cation sorption on clays.