Intensity dependent transmission and laser-induced fluorescence were observ
ed in liquid solutions of mesoionic compounds (MIC) pumped with nanosecond
lasers operating at 1064, 604, and 570 nm. The results indicate that two-ph
oton absorption (TPA) is the dominant mechanism which causes the observed b
ehavior. The TPA cross-sections measured have values from 0.33 x 10(-20) cm
(4)/GW to 0.43 x 10(-18) cm(4)/GW. (C) 2000 Elsevier Science B.V. All right
s reserved.