Electronic energy transfer in a microcavity

Citation
Dm. Basko et al., Electronic energy transfer in a microcavity, PHYS REV B, 62(23), 2000, pp. 15962-15977
Citations number
39
Categorie Soggetti
Apllied Physucs/Condensed Matter/Materiales Science
Journal title
PHYSICAL REVIEW B
ISSN journal
01631829 → ACNP
Volume
62
Issue
23
Year of publication
2000
Pages
15962 - 15977
Database
ISI
SICI code
0163-1829(200012)62:23<15962:EETIAM>2.0.ZU;2-U
Abstract
We study the microcavity effect on energy transfer via the electromagnetic field. The modification of the optical propel ties of the microcavity due t o the presence of absorbing accepters is taken into account. We analyze dif ferent cases that may be realized depending on the characteristics of the a cceptor absorption band: the case of strong and broad absorption, when the cavity mode is practically destroyed; the regime of weak absorption, when t he cavity mode is still well defined and just acquires some additional broa dening; and the strong-coupling regime, when the acceptor absorption has th e shape of a strong and narrow peak and two polariton branches appear, form ed due to coherent mixing of the acceptor excitations and the cavity mode. In our calculations we use a realistic model for the cavity mirrors (dielec tric or metallic), which is important since the mirrors introduce an additi onal decay channel for the donor excitation besides the transfer to the acc epters. The distribution of the energy between different decay channels is analyzed in detail.