ArF excimer laser ablation of micrometer size smoke grains was investigated
. It was demonstrated that this procedure is suitable for destruction of th
ese particulates in consequence of very fast heating, oxidation, burning, a
nd evaporation. The time-resolved investigations revealed that the destruct
ion process takes place between 0 and 7 ns after the maximum of the excimer
pulse. The efficiency of breaking into small pieces was found to be depend
ent on the excimer laser fluence. Atomic force microscopic investigations o
f the sedimented smoke particles proved that the size of the grains signifi
cantly decreased by the excimer laser radiation. (C) 2001 American Institut
e of Physics.