The temporal and spectral properties of two-photon induced fluorescence and
up-conversion lasing of two new laser dyes have been experimentally invest
igated. Pumped by 1064 nm mode-locked Nd:YAG laser, effective two-photon in
duced fluorescence with peak wavelength at 635 nm and up-conversion lasing
at similar to 626 nm emitted from the solutions of these new dyes in DMF. T
he lifetimes of two-photon up-conversion fluorescence of the two dyes are 6
5 and 67 ps. At picosecond laser pumping, the efficiency of up-conversion l
asing is 8.4% and 9.1% for the two new dyes. (C) 2001 Elsevier Science B.V.
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