Giant optical responses in microcavity-fractal composites

Citation
Va. Podolskiy et Vm. Shalaev, Giant optical responses in microcavity-fractal composites, LASER PHYS, 11(1), 2001, pp. 26-30
Citations number
31
Categorie Soggetti
Apllied Physucs/Condensed Matter/Materiales Science","Optics & Acoustics
Journal title
LASER PHYSICS
ISSN journal
1054660X → ACNP
Volume
11
Issue
1
Year of publication
2001
Pages
26 - 30
Database
ISI
SICI code
1054-660X(200101)11:1<26:GORIMC>2.0.ZU;2-Y
Abstract
Optical properties of fractal nanostructured composite materials are consid ered. The fractal geometry results in localization of plasmon excitations i n the "hot" spots, where the local field can exceed the applied field by se veral orders of magnitude. The high local fields of the localized fractal m odes result in dramatic enhancement of optical responses, making feasible t he surface-enhanced nonlinear spectroscopy of single molecules and nanocrys tals. The field enhancement becomes especially large when fractals are plac ed inside a microcavity. A theory for the enhanced Raman and hyper-Raman su rface-enhanced scattering in microcavity-fractal composites is developed.