Is contrast to the experimentally widely used isentropic demagnetization pr
ocess for cooling to ultra-low temperatures we examine a particular classic
al model system that does not cool, but rather heats up with isentropic dem
agnetization. This system consists of several magnetite particles in a coll
oidal suspension, and shows the uncommon behavior of disordering structural
ly while ordering magnetically in an increasing magnetic field. For a six-p
article system, we report an uncommon structural transition from a ring to
a chain as a function of magnetic field and temperature.